Neutron and Gamma-Ray Spectra from 232Th, 235U, 238U, and 239Pu After Bombardment with 14-MeV Neutrons

Abstract
The neutron and gamma-ray leakage spectra from pulsed spheres having a radius equal to 1.0 mean-free-path (mfp) for 14-MeV neutrons in 232Th, 235U (with radii of 0.7 and 1.5 mfp), 228U (with radii of 0.8 and 2.8 mfp), and 239Pu (with radii of 0.7 and 1.25 mfp) were measured by using time-of-flight techniques. The neutron spectra were measured between 0.9 and 15 MeV using stilbene and NE-213 scintillators. For the gamma rays, the electron recoil spectra were measured between 0.35 and 8 MeV with the NE-213 detector only. Pulse-shape discrimination and flight paths of ∼10 m were used in these measurements. The measured spectra are compared with calculations carried out with TARTNP, a coupled neutron-photon Monte Carlo transport code. The Lawrence Livermore Laboratory ENDL (neutron and photon cross sections) and ENDF/B-IV libraries were used in these calculations.In the region between 10 and 15 MeV, the calculated neutron spectra are in good agreement with the measurements (±5%). The maximum discrepan...

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