Quantum tunneling and classical barrier reduction for a mesoscopic spin
- 1 May 1998
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 57 (17) , 10291-10294
- https://doi.org/10.1103/physrevb.57.10291
Abstract
I show that for a large spin with uniaxial anisotropy it is, in principle, impossible to distinguish classical energy-barrier reduction due to a transverse magnetic field from an increase in the tunneling rate of excited levels. Given a suitable definition of the quantum energy barrier, I derive an expression for the field dependence of the barrier height that agrees with the classical result up to a constant of order unity. Numerical results show that for a mesoscopic spin the barrier decreases in a series of steps, which recent experiments may have revealed.
Keywords
This publication has 20 references indexed in Scilit:
- Single-Molecule Magnets: Magnetization Relaxation and Quantum Tunneling in Dodecanuclear Manganese ComplexesMolecular Crystals and Liquid Crystals, 1997
- Quantum Tunneling of the Magnetization in an Iron Cluster NanomagnetPhysical Review Letters, 1997
- Effect of a transverse magnetic field on resonant magnetization tunneling in high-spin moleculesJournal of Applied Physics, 1997
- Thermally assisted macroscopic quantum resonance on a single-crystal of Mn12-acetateJournal of Applied Physics, 1997
- Evidence for resonant tunneling of magnetization insacetate complexPhysical Review B, 1997
- Macroscopic quantum tunnelling of magnetization in a single crystal of nanomagnetsNature, 1996
- Field tuning of thermally activated magnetic quantum tunnelling in Mn 12 − Ac moleculesEurophysics Letters, 1996
- Macroscopic Measurement of Resonant Magnetization Tunneling in High-Spin MoleculesPhysical Review Letters, 1996
- Steps in the hysteresis loops of a high-spin moleculeJournal of Applied Physics, 1996
- Mesoscopic quantum tunneling of the magnetizationJournal of Magnetism and Magnetic Materials, 1995