Low-Temperature Quantum Relaxation in a System of Magnetic Nanomolecules
Preprint
- 23 October 1997
Abstract
We argue that to explain recent resonant tunneling experiments on crystals of Mn$_{12}$ and Fe$_8$, particularly in the low-T limit, one must invoke dynamic nuclear spin and dipolar interactions. We show the low-$T$, short-time relaxation will then have a $\sqrt{t/\tau}$ form, where $\tau $ depends on the nuclear $T_2$, on the tunneling matrix element $\Delta_{10}$ between the two lowest levels, and on the initial distribution of internal fields in the sample, which depends very strongly on sample shape. The results are directly applicable to the $Fe_8$ system. We also give some results for the long-time relaxation.
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All Related Versions
- Version 1, 1997-10-23, ArXiv
- Published version: Physical Review Letters, 80 (26), 5794.
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