The Structure of Gaseous 2-Azetidinone as Studied by Microwave Spectroscopy, Electron Diffraction, and Ab Initio Calculations.

Abstract
The simplest four-member .beta.-lactam, 2-azetidinone, has been studied by microwave spectroscopy, electron diffraction and ab initio quantum chemical computations at the 6-31G** level. An accurate rg structure has been determined by making use of rotational constants from five isotopic species and electron diffraction data in a joint analysis. The molecule is planar (apart from the methylene group hydrogen atoms) in the gas phase. The dipole moment and 14N quadrupole coupling constants have been determined. Numerous vibrationally excited states have also been assigned for the parent and one deuterated species. The ring-puckering potential was determined from the vibrationally excited states of the puckering vibration.

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