Impedance Model for a Concentrated Solution: Application to the Electrodissolution of Copper in Chloride Solutions

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Abstract
From the Stefan‐Maxwell equations, a model has been developed which describes the distribution of concentration of each species in the solution. This model has provision for an arbitrary number of simultaneous homogeneous and heterogeneous reactions and is used to treat the steady state and the impedance of an electrochemical interface. As an example, this method is applied to the anodic dissolution of a rotating disk of copper in chloride solutions.

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