Two-photon processes in real atoms

Abstract
We present a general method for calculating two-photon processes in real atoms by a variant of the usual multichannel quantum-defect theory (MQDT). Most notably, this method enables us to describe processes in which a single photon has enough energy to ionize the atom (above-threshold processes). All effects of intermediate Rydberg series, continua, or autoionizing series are treated on an equal footing and with the same ease; the final state is also treated properly by standard MQDT. This method should also work for many three- or four-photon processes.

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