Random-field-induced destruction of the phase transition of a diluted two-dimensional Ising antiferromagnet: Rb2Co0.85Mg0.15F4

Abstract
Optical birefringence has been used to study the effects of a uniform field H on the magnetic specific heat Cm near the phase transition of a randomly diluted, two-dimensional (2D) Ising antiferromagnet, Rb2 Co0.85 Mg0.15 F4. For H=0, a well-defined transition is observed with a symmetric logarithmic divergence in Cm, corresponding to the critical exponent α=0, as is predicted for the 2D Ising random-exchange case. With H applied parallel to the c axis, a systematic rounding of the peak in Cm occurs which increases with increasing H. This demonstrates that induced random fields destroy the phase transition and that the lower critical dimensionality for the random-field problem dl2. No rounding is found with Hc, as expected. The peak in Cm with Hc exhibits a decrease in amplitude, which varies as lnH. This behavior, together with the ln |t| dependence of Cm at H=0, was used to determine the crossover exponent φ=1.58±0.22. This value is in essential agreement with the exactly known critical exponent of the staggered susceptibility γ for the 2D Ising problem, namely γ=74, as predicted theoretically. By suitable rescaling, the rounded peaks found for different values of H may all be collapsed to a single curve in the critical region, in accord with renormalization-group scaling relations. The shift and rounding (and hence the peak amplitude) are in quantitative agreement with the site-diluted, random-field predictions.