Coexistence of Antiferromagnetism and Superconductivity: A Neutron Diffraction Study of DyMo6S8

Abstract
Although DyMo6 S8 is a superconductor below Tc=2.05 K previous studies of the resistivity, susceptibility, and upper critical field strongly suggest the development of magnetic order at TM=0.4 K. The present neutron study shows conclusively that this superconducting compound also develops coexistent long-range (greater than 300 Å) antiferromagnetic order at TM. The Dy atoms form a simple cubic sublattice (with a slight rhombohedral distortion) in which the observed magnetic structure consists of (100) planes with moments of 8.77μB alternately parallel and antiparallel to the [111] direction.