The diazonium group: an electron acceptor for large molecular hyperpolarizabilities

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Abstract
The diazonium compounds 4-dialkylamino-4′-phenylazobenzenediazonium tetrafluoroborate are synthesised and their molecular hyperpolarizabilities (β) measured with the hyper-Rayleigh scattering technique; the diazonium compounds show much larger β values than the corresponding nitro compounds.

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