Colorimetric Determination of Allyl Isothiocyanate

Abstract
A simple and accurate colorimetric method for determination of allyl isothiocyanate was developed. It involves formation of methylene blue by the reaction of an acid solution of N, N-dimethyl-p-phenylenediamine in the presence of ferric ion with the sulfide liberated by ethanolic base hydrolysis of allyl isothiocyanate in xylene. This method permits determination of microgram quantities of S in allyl isothiocyanate. The effects of alterations in reaction conditions on the color development were investigated. Tests with a range of sulfur-containing organic compounds (thiourea, cysteine, methionine, cysteic acid, thioacetamide, benzene sulfonamide, glucose-6-Sulfate, and sinigrin) showed that none of the compounds tested interfere with this method when the S concentration is ≤ 10 times that of S as allyl isothiocyanate.

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