Isotope scattering of dispersive phonons in Ge

Abstract
With the use of a lattice-dynamical model which reproduces observed phonon dispersion curves very accurately, the isotope scattering of near-zone-boundary acoustic phonons in Ge is investigated theoretically. We show that the lattice dispersion which becomes appreciable in the THz-frequency region leads to the phonon relaxation time that decreases more rapidly than ω4. This deviation from the ω4 dependence (the ω4 behavior is predicted by the continuum elasticity theory) amounts to about 20% at 1 THz and is enhanced heavily at the zone boundaries. Calculations are based on the lowest-order perturbation theory. Higherorder corrections are estimated as well and shown to be negligibly small.