Two New Standards for the pH Scale.

Abstract
Two new primary standards for the NBS pH scale, supplementing the five already available, are proposed. The new reference solutions are the 0.05 molal solution of potassium dihydrogen citrate and a mixture of sodium bicarbonate and sodium carbonate, each 0.025 molal. The citrate solution has a pH of 3.776 at 25 °C and is more stable under certain conditions than either the tartrate or phthalate standards. The carbonate solution has a pH of 10.012 at 25 °C. It therefore extends the NBS pH scale above its present upper limit of 9.180 at this temperature. Reference values pH(S), based on emf measurements of cells with hydrogen electrodes and silver-silver chloride electrodes, have been assigned to these two standard solutions at 11 temperatures from 0 to 50 °C.

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