Improved Preparation of 5,6-Dialkoxy-1,1-dimethylindenes, Precocene Analogues Lacking the Pyranyl Oxygen Atom [1]

Abstract
The use of methanesulfonic acid as solvent and catalyst in the cyclocondensation of 1,2-dialkoxybenzenes with 3-methylbut-2-enoyl chloride to afford indanones 3, thus allowing the preparation of indenes 4 with improved overall yields, is reported. Additionally, structure of dimeric compound 7 a, formed in high yield by thermal treatment of 4a has been determined by com bination of spectroscopic means and selective deuterations.

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