Reduction of adenine dihydrochloride by ionizing radiation

Abstract
The reduction product produced by ionizing radiation in single crystals of adenine dihydrochloride x irradiated at 4.2 °K was studied by ESR–ENDOR spectroscopy. Addition of an electron to the protonated base yields a free radical with a spin density of approximately 0.30 on the C‐8 carbon atom. The spin density was inferred from ENDOR measurements of the hyperfine coupling of the C8–H proton.

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