De novo design of microporous transition metal oxides

Abstract
Ab initio Hartree–Fock calculations are performed on the molybdenum and tungsten trioxides and bronzes, obtained by inserting alkali metal atoms or larger species in the MO3 framework; we examine four known polymorphs and two new structures with a microporous architecture, and characterise their relative stability; we also explore the synthesis conditions under which the microporous polymorphs may be obtained, by designing potential organic templates.

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