Synthesis of a new organic π-donor: 2-(thiopyran-4-ylidene)-1,3-dithiole and its conducting salts with 7,7,8,8-tetracyanoquinodimethane

Abstract
The new organic π-donor, 2-(thiopyran-4-ylidene)-1,3-dithiole (3), iso-π-electronic to both tetrathiafulvalene (1) and Δ4,4′-bithiopyran (2) and obtained by a three-step synthesis in 15% overall yield, reacts with 7,7,8,8-tetracyanoquinodimethane (TCNQ) to give two semiconducting salts.

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