Abstract
From the reaction of silylated 4-(3,3-dimethyl-1-triazeno)imidazole-5-carboxamide (DTIC, 5) and 3-(3,3-dimethyl-1-triazeno)pyrazole-4-carboxamide (DTPC, 9) with 2-chlorotetrahydrofuran, in both cases a single tetrahydrofuran-2-yl derivative was isolated. When silylated DTPC was reacted with 2-chlorotetrahydropyran, 2 tetrahydropyran-2-yl compounds were obtained. These were shown to be positional isomers on the basis of 1H NMR and UV data. These furanyl and pyranyl derivatives were tested for antileukemic activity ([mouse] L-1210, in vivo) and the results were compared with the results obtained for the corresponding ribosyl derivatives of DTIC and DTPC.

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