Self-Consistent-Field Theory. II. The LCAO Approximation

Abstract
In Part I of this series, eigenvalue equations which apply to any electronic system were developed by means of a general coupling operator. These equations are here adapted to the method of linear combinations of atomic orbitals. The resultant matrix equations are applied to the helium atom for the configurations: 1S, (1s)2; 3S, (1s) (2s); 1S, (1s) (2s), using Slater 1s and 2s orbitals as basis functions.

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