Interplay between charge, orbital and magnetic order in Pr_{1-x}Ca_xMnO_3
Preprint
- 19 May 1999
Abstract
We report resonant x-ray scattering studies of charge and orbital order in Pr_{1-x}Ca_{x}MnO_3 with x=0.4 and 0.5. Below the ordering temperature, T_O=245 K, the charge and orbital order intensities follow the same temperature dependence, including an increase at the antiferromagnetic ordering temperature, T_N. High resolution measurements reveal, however, that long range orbital order is never achieved. Rather, an orbital domain state is formed. Above T_O, the charge order fluctuations are more highly correlated than the orbital fluctuations. Similar phenomenology is observed in a magnetic field. We conclude that the charge order drives the orbital order at the transition.Keywords
All Related Versions
- Version 1, 1999-05-19, ArXiv
- Published version: Physical Review Letters, 83 (23), 4872.
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