Nitroalkenylferrocene. III. Condensation Reaction of Acetylferrocene Using Lewis Acid and Cyclic Amine

Abstract
Acetylferrocene reacted with nitromethane and morpholine in the presence of titanium(IV) chloride to give a Mannich base, 2-ferrocenyl-2-morpholino-1-nitropropane (7), whose sodium salt (8) was then converted to 2-ferrocenyl-1-nitropropene (9) by acidifying it with hydrochloric acid. In the presence of aluminum chloride in place of titanium (IV) chloride, acetylferrocene as well as 1,1′-diacetylferrocene dimerized to form α,β-unsaturated ketone, (10) or (11).

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