The transient operation of a solid oxide fuel cell monolith under forced periodic reversal of the flow
- 1 October 1996
- journal article
- research article
- Published by Wiley in The Canadian Journal of Chemical Engineering
- Vol. 74 (5) , 719-728
- https://doi.org/10.1002/cjce.5450740523
Abstract
The forced periodic reversal of the flow is proposed for the case of a Solid Oxide Fuel Cell (SOFC) monolith. A one‐dimensional non‐steady state heterogeneous model is applied to an investigation of H2 electrochemical oxidation in a co‐current flow solid oxide monolithic fuel cell. Results are reported on the transient evolution along the reactor, of the species conversion, temperature distribution, thermodynamic energy conversion efficiency and volumetric power density. This novel transient operation of an SOFC leads to improved and highly efficient performances, thus allowing for a combination of the concepts of a regenerative heat preheater and of an electrocatalytic converter, in a single SOFC monolithic assembly.Keywords
This publication has 15 references indexed in Scilit:
- A bench scale study of reversed flow methanol synthesisIndustrial & Engineering Chemistry Research, 1992
- Performance of catalytic processes under unsteady conditionsChemical Engineering Science, 1990
- Mathematische Modellierung chemischer Reaktoren — Entwicklung und Einbindung neuer TechnologienAngewandte Chemie, 1990
- Chemical Cogeneration in Solid Electrolyte Cells: The Oxidation of toJournal of the Electrochemical Society, 1990
- Wellenausbreitung in verfahrenstechnischen ProzessenChemie Ingenieur Technik - CIT, 1989
- Catalytic combustion with periodic flow reversalChemical Engineering Science, 1988
- Steady-state analysis of high temperature fuel cellsChemical Engineering Science, 1983
- Ammonia oxidation to nitric oxide in a solid electrolyte fuel cellSolid State Ionics, 1981
- Overpotential Behavior of Stabilized Zirconia Solid Electrolyte Fuel CellsJournal of the Electrochemical Society, 1971
- Westinghouse Solid-Electrolyte Fuel CellPublished by American Chemical Society (ACS) ,1969