[CoII2L(NCS)2(SCN)2]: The First Cobalt Complex to Exhibit Both Exchange Coupling and Spin Crossover Effects

Abstract
A spin crossover transition (350 K, μeff=3.15 μB per Co atom; 4.5 K, μeff=0.70 μB per Co atom) and weak antiferromagnetic exchange (2 J=−11.7 cm−1) between the octahedral, doubly pyridazine bridged cobalt(II) ions are features of the structurally characterized complex [CoII2L(NCS)2(SCN)2] (the ligand L is shown).

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