New spin-fluctuation system:U0.5Th0.5Al3

Abstract
Low-temperature measurements show a T3(lnT/TSF) term in the specific heat of the pseudobinary compound U0.5 Th0.5 Al3. This is considered strong evidence for long-range ferromagnetic spin fluctuations. The specific heat γ is 360 mJ/[(mole U) K2] and χ(T→0)=9.6×103 emu/(mole U). Except for a much less rapid decrease in resistance below 50 K than in UPt3, the resistance, susceptibility, and specific-heat data for the D019 structure U0.5 Th0.5 Al3 are very similar to those of the isostructural heavy-fermion superconductor UPt3. In addition to the poorer resistivity ratio, U0.5 Th0.5 Al3 has a significantly larger (∼50%) Wilson ratio than UPt3, explaining the lack of superconductivity down to 0.020 K.