Abstract
Oxidation of cis-[RuII(6,6′-Cl2bpy)2(OH2)2]2+ with CeIV gave cis-[RuVI(6,6′-Cl2bpy)2O2]2+, isolated as the diamagnetic ClO4 salt, which rapidly oxidizes Cl(to Cl2) and a wide variety of organic substrates (tetrahydrofuran to butyrolactone and cyclohexane to cyclohexanone).

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