Abstract
A steady-state computer-simulation method is described for the calculation of the chemical diffusion coefficient in the pseudo-one-component lattice gas with nearest-neighbour interactions. This formalism provides a useful framework for describing the important configurational aspects of diffusion in interstitial solid solutions and non-stoichiometric compounds. The results for the chemical diffusion coefficient are in excellent agreement with the exact modified Darken equation using independently obtained simulated values of the self-diffusivity, physical correlation factor and the chemical potential.