Magnetic circular dichroic effects in the luminescence ofcenters in KI, KBr, and KCl
- 15 December 1977
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 16 (12) , 5570-5584
- https://doi.org/10.1103/physrevb.16.5570
Abstract
We have measured magnetic-field-induced circular polarization of the -center emission in Kl, KBr, and KCl at 1.9 K in fields up to 80 kG. Both diamagnetic (field-dependent) and paramagnetic (spin-dependent) effects have been observed. The latter requires a special technique in which the pump beam is modulated between right and left circular polarization. The expected behavior as a function of the frequency of the modulation has been observed. We have also measured the spin-lattice relaxation time in the relaxed excited state in KI and KBr for kG. All the previous measurements indicate a value of the spin-orbit splitting, , of the order of 1 meV, which is considered a surprisingly small value from purely theoretical grounds.
Keywords
This publication has 25 references indexed in Scilit:
- Vibronic Problem for the Relaxed Excited State of the F-center in Alkali Halides. II. Analysis of the ExperimentsJournal of the Physics Society Japan, 1976
- Vibronic Problem For the Relaxed Excited State of the F-center in Alkali Halides. I. Vibronic Energy SchemesJournal of the Physics Society Japan, 1976
- Nonlinear Optical Excitation of the Relaxed Vibronic States of theCenter in KC1Physical Review Letters, 1975
- A contribution to the discussion on the relaxed excited F centrePhysica Status Solidi (b), 1975
- Infrared Absorption Spectrum of the Relaxed Excited State of theCenter in Potassium HalidesPhysical Review Letters, 1975
- The Influence of “Rotational” Lattice Deformation States on the F Center EmissionPhysica Status Solidi (b), 1974
- Relaxed Excited States of theCenter: A Study of the Nearly Degenerate States of a Bound Lattice PolaronPhysical Review B, 1973
- Empirically Determined Wave Function for the Relaxed-Excited State of theCenter in KIPhysical Review Letters, 1972
- Dynamical Jahn-Teller effect in relaxed excited state of F-centerJournal of Physics and Chemistry of Solids, 1972
- Stark Effects in-Center EmissionPhysical Review B, 1970