A Concise Synthesis of (+)-(S)-Dihydroperiphylline

Abstract
The total synthesis of the spermidine alkaloid, (+)-(S)-dihydroperiphylline, is described. The key reactions in the present strategy are enantioselective aldol-type reaction of imines with ketene silyl acetals promoted by chiral BLA (Brønsted acid assisted chiral Lewis acid) and boron-templated cyclization of triamino esters.

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