Nonadiabatic Effects in the Internal Rotation of ·CH2COO− in Irradiated Zinc Acetate Dihydrate

Abstract
The article of record as published may be found at http://dx.doi.org/10.1063/1.1673974The EPR spectrum of the • CH2Coo- radical in a single crystal host displays nonadiabatic motional effects. A phenomenological theory is suggested, based on the density matrix of the spin system, and a technique is described for rapid calculation of simulated spectra.Office of Naval Researc