Time Correlation Functions for Internal and Anisotropic Rotational Motion of Molecules

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Abstract
By use of Green's functions for the diffusional motion a very concise formulation and computation of correlation functions is possible. For an axially symmetric overall diffusion with internal rotation about one and two axes correlation functions of a second rank spherical tensor are calculated. The results comprise all the solutions of the pertinent problem as given so far and allow the extension of the theory to a wider field of application

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