Reaction of α-metallated N-acyl-λ5-phosphazenes with aryl cyanides

Abstract
Metallated N-acyl-λ5-phosphazenes react with aryl cyanide to give imino-λ5-phosphazenes (6) and (7), in which nitrite insertion into the phosphorus–carbon bond of N-acyl-λ5-phosphazenes (2) and (3) takes place. Subsequent reactions of the imino- and enamino-N-ethoxycarbonyl-λ5-phosphazenes (7) and (9) afford the phosphine oxide derivatives (13) and (11), through a cyclocondensation and hydrolysis sequence.

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