La139NQR relaxation and μSR study of Zn-doping effects inLa2CuO4

Abstract
La139 NQR and zero-field μ+SR in antiferromagnetic (AF) La2 Cu1x Znx O4, for x up to 0.13 and in the temperature range 1.6–350 K, are used to study the effects related to the substitution of magnetic Cu2+ S=1/2 with homovalent diamagnetic S=0 Zn2+ in La2 CuO4. We report measurements both of static magnetic properties, such as Néel temperatures TN, sublattice magnetization and field ‖h‖ at the La nucleus or at the μ+ site, as well as of NQR relaxation rates W. These quantities are used to study the effects of Zn doping on the low-energy Cu2+ spin excitations. It is found that TN decreases with x in a way close to the one expected by diluting quasi-two-dimensional Heisenberg magnets on square lattice, while the sublattice magnetization is slightly affected by Zn doping. Mean-field arguments based on the dilution model for the interplanar interactions allow one to conclude that the in-plane magnetic correlation length is little sensitive to the Zn presence. Up to x≃0.08 the temperature dependence of the AF field ‖h‖ is close to the one in pure La2 CuO4, with a sharp decrease for TTN indicative of a continuous transition with a small critical exponent β.