Two photon laser spectroscopy of indium

Abstract
Two photon transitions from the 52P0½and 52P03/2states of In have been observed to high lying2P0and2F0states. Extended series corresponding to P0nP0and P0nF0transitions are seen ton= 23 andn= 31 res­pectively. A hybrid resonance through intermediate states of In2gives rise to a series 6s2S →np2P0which can be followed ton= 42. Resonant en­hancement of the 52P03/2np2P0series occurs because of an intermediate2S state. This produces a singularity in the cross section for this transition. Possible two photon transitions to autoionizing states of In are also seen.

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