Abstract
Three intermediates in the acid hydrolysis of [Cr(CN)5NO]3– are detected in solution by e.s.r. at room temperature, the final product being [Cr(NO)(H2O)5]2+. Each species is characterised by different A(14N), A(53Cr), or g values. Kinetics of the last two stages of the reaction have been studied to determine the dependence of reaction rates on acid concentration and to evaluate the activation parameters.

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