Raman scattering from spin fluctuations in , , and
- 1 February 1991
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review B
- Vol. 43 (4) , 3009-3019
- https://doi.org/10.1103/physrevb.43.3009
Abstract
Antiferromagnetic excitations in single crystals of , , and were investigated as a function of Ce concentration using Raman scattering at room temperature. The introduction of electrons by Ce doping significantly broadens the two-magnon peak in the mode, indicating that zone-boundary magnons become damped with increasing Ce concentration. The existence of broad spin-pair-excitation spectra in the and modes at x=0.15 suggests that the short-range spin fluctuations persist in these electron-doped superconductors. The energy of the spin-pair-excitation peak in is not affected by doping up to x=0.2. This is similar in behavior to the system up to x=0.17. The absence of softening of the short-wavelength magnons in these systems is in marked contrast to the magnon softening behavior in . The Raman spectra in make no distinction between the superconducting and the metallic regions. The highly damped magnetic-excitation spectra support the picture that the spin-spin correlation length in the present systems decreases gradually with increasing Ce concentration.
Keywords
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