Soft-sphere model for the glass transition in binary alloys. II. Relaxation of the incoherent density-density correlation functions
- 1 July 1988
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review A
- Vol. 38 (1) , 454-462
- https://doi.org/10.1103/physreva.38.454
Abstract
Using molecular-dynamics (MD) data on a binary-alloy model, we have computed the self (incoherent) -part of the density autocorrelation functions of both species in the supercooled liquid and near the glass transition, over an extensive range of wave numbers. Standard theoretical models of liquid-state theory fail to reproduce the data, while the Chudley-Elliott jump diffusion model yields reasonable results in the glass range. With a suitable scaling of the time axis, the data for different temperatures can be brought onto a single master curve, which is well fitted by a Kohlrausch (‘‘stretched-exponential’’) function with a wave-number-dependent exponent.Keywords
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