Neutron diffraction study of magnetically ordered Tm2Fe3Si5

Abstract
Tm2 Fe3 Si5 has been studied at low temperatures by neutron powder diffraction techniques. At T=1.5 K the diffraction pattern is characteristic of a tetragonal crystal structure, space group P4/mnc (D4h6; with a=10.332 Å and c=5.388 Å), similar to that of the prototype compound Sc2 Fe3 Si5. Below T=1.2 K magnetic scattering peaks develop, which can be indexed with the parameters of the chemical cell. A noncollinear antiferromagnetic structure is proposed which features ordering of Tm moments in the 〈110〉 set of directions. The magnetic moment of Tm is 6.5μB at the lowest temperature attained, 0.35 K.