Fluctuation-Dominated Kinetics under Stirring
Open Access
- 27 January 1997
- journal article
- research article
- Published by American Physical Society (APS) in Physical Review Letters
- Vol. 78 (4) , 741-744
- https://doi.org/10.1103/physrevlett.78.741
Abstract
We investigate the effects of stirring on the kinetics of the reaction under stoichiometrical conditions in 2D. We consider both a steady eddy-lattice flow and a random flow mimicking turbulence. In both situations complex decay patterns are detected. Only an intermediate stage of the reaction is dominated by mixing. The long-time behavior shows fluctuation-dominated kinetics, , governed by effective diffusion. For the case of an eddy-lattice flow a very slow intermediate regime emerges, , which is associated with the closed topology of flow lines.
Keywords
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