Critical behavior of the spontaneous magnetization at marginal dimensionality in LiHoF4

Abstract
We have measured the critical behavior of the spontaneous magnetization as a function of temperature for T<~Tc in the three-dimensional, uniaxial, dipolar-coupled ferromagnet LiHoF4 using elastic-laser-light-scattering techniques. In the reduced-temperature range 1.3×103<~t<~1.3×101, we find that the logarithmically corrected mean-field power law M(T)M(0)=Bt12|ln|t0t||13 fits the data with Tc=1.5383±0.0003 K, t0=0.483±0.046, and χ2=1.34. We have also fitted the data to M(T)M(0)=B|t|12|ln|t||13[1+C1(ln|ln|t||ln|t|)+C2(1ln|t|)] in order to obtain explicitly the corrections to the leading singularities. We find in this fit that Tc=1.5382±0.0003 K, C1=0.07±0.3, C2=0.287±0.07, and χ2=1.26. Fits to a simple power law M(T)M(0)=Btβ yield Tc=1.5370±0.0002 K, β=0.355±0.005, and χ2=17.2. We also present measurements of the temperature and magnetic-field dependence of the light scattering in LiHoF4, and the magnetic-field and wavelength dependence of the circular birefringence.