Inelastic neutron scattering measurements on [Cu4OCl6L4] (L = pyridine or dimethyl sulfoxide). Observation of zero-field splitting of the cluster ground state

Abstract
Inelastic neutron scattering measurements on the complexes [Cu 4 OCl 6 L 4 ] (L = pyridine or dimethyl sulfoxide) revealed ground-state zero-field splittings of ca. 3 and 6 cm -1 . The splittings are interpreted as due to the combined effects of exchange and spin–orbit coupling, and suggest a new interpretation of previous magnetic data.

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