Abstract
The crystal structure of the reversible dioxygen adduct of [N,N′-(3,3′-dipropylmethylamine)bis(salicylideneaminato)cobalt(II)](1), crystallized from benzene, shows the presence of both dioxygenated and non-dioxygenated monomric molecules containing, respectively, low-spin octahedral and high-spin five-co-ordinated cobalt atoms.

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