Abstract
The values 1J(15N≡13C) from 15N satellites in the 13C NMR spectra for two nitriles [C6H5-C≡N, (CH3)2CH-C≡N] have been determined and δ(15N) for trimethylsilylcyanide has been con- firmed. This completed a set of NMR parameters in order to compare phosphaalkynes and nitriles. Linear relationships emerged for the following NMR parameters of phosphaalkynes and nitriles: δ(31Pp≡c)/δ(15NN≡C), δ(13CP≡C)/δ(13CN≡C) and 1J(31P=13C)/1J(15N≡13C). On the basis of the latter relationship a positive sign for 1J(31P≡13C) has been proposed. This is also corroborated by the sub- stituent-induced changes in the magnitude of 1J(13C≡13C) in corresponding alkynes.

This publication has 0 references indexed in Scilit: