Unusually slow temporal evolution of femtosecond four-wave-mixing signals in intrinsic GaAs quantum wells: Direct evidence for the dominance of interaction effects

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Abstract
Four-wave-mixing signals from excitons in high-quality GaAs quantum wells show an unusually slow temporal evolution, in stark contrast to the behavior expected for a noninteracting two-level system. We show that Coulomb interaction effects, generally neglected in the analyses of four-wave-mixing experiments, dominate the signals by 2 orders of magnitude. Numerical calculations based on extended optical Bloch equations for semiconductors provide good qualitative agreement with the data.