Quantum spin liquid: The Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice

Abstract
We calculate the correlation functions of the S=12 Heisenberg antiferromagnet on the three-dimensional pyrochlore lattice. We use a perturbative expansion in terms of spin blocks. This method is self-controlled by the extracted correlation length. We find that the ground state is a spin-liquid state: the spin-spin correlation functions decay exponentially with distance and the correlation length never exceeds the interatomic distance, even at T=0. The static structure factor becomes dispersive, indicating a selection of modes by thermal and quantum fluctuations. We also calculate the magnetic neutron diffraction cross section in two planes of the reciprocal space and we find a very good agreement with neutron experiments performed on Y(Sc)Mn2 and CsNiCrF6.