Fractional Quantization of Molecular Pseudorotation inNa3

Abstract
Fractional quantization of the adiabatic pseudorotation in an isolated molecule is reported. This result, concerning the large-amplitude pseudorotation in 22ENa3, constitutes the first direct verification of the adiabatic sign-change theorem, and also presents the most complete picture of the level structure and internuclear dynamics of a metal-atom cluster yet given.

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