Abstract
The novel 5-exo-phosphino-η4-cyclopentadienyl complexes (η4-C5H5PR1R2)Fe(CO)3 (4) (a: R1=R2=SiMe3; b:R1=t-Bu; R2=SiMe3) are obtained by the nucleophilic addition of LiPR1R2 to the carbocyclic ligand in [(η5-C5H5)Fe(CO)3]PF6. At room temperature 4a, b are converted into (η5-C5H5)(CO)2Fe-PR1R2 (5a, b).

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