13C CPMAS NMR spectra of solid proton-exchanging p-substituted benzoylacetones: observation of13C,35,37Cl residual dipolar coupling in the p-chloro derivative

Abstract
Residual dipolar coupling to spin-3/2 35,37Cl nuclei appears as a symmetric doublet of 0.69 kHz in the 13C CPMAS NMR spectrum of p-chlorobenzoylacetone at 75.4 MHz, in agreement with theoretical calculations; carbon chemical shifts of a series of p-substituted benzoylacetones undergoing solid proton transfer are also reported, which show tautomeric populations similar to the solution ones.

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