EuAl2at pressures up to 41 GPa: A localized magnet exhibiting highly nonlinear electronic effects

Abstract
Eu151 Mössbauer studies under hydrostatic pressures up to 41 GPa coupled to x-ray diffraction measurements show that—contrary to expectations—the 4f electrons in EuAl2 remain fully localized even under a reduction of unit cell volume of ∼30%. However, strongly nonlinear effects are observed for the conduction electron polarization, for the s-electron density ρ(0) at the Eu151 nucleus, the Néel temperature TN, and the transferred hyperfine field hyperbolically; TN and Bthf connected to ρ(0). The latter results can be described quantitatively within the RKKY formalism.