Truncated expansion of the ground-state energy of a neutral atom in powers of Z-1/3: coefficients of the leading terms

Abstract
Numerical estimates of the ground-state energy E of a neutral atom of atomic number Z have been obtained for a few values of Z ranging from 86 to 290 by performing atomic self-consistent-field calculations, treating exchange exactly, using a statistical approximation for correlation, and neglecting relativistic corrections. These numerical values are used to estimate the coefficients in a truncated expansion of E in powers of Z-13/. Writing E approximately=-(c7Z7/3+c6Z6/3+c5Z5/3+c4Z4/3)Ryd with c7 determined from the Thomas-Fermi model the authors find c6=-1.0 in agreement with the prediction of Scott (and of Lieb (1976) and of Schwinger (1980)), they find c5 approximately=0.55, which is close to the value suggested by March and Plaskett, and they find that c4, if it exists, is near to zero.

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