Etude spectroscopique des dérives du peroxyde d'hydrogène. II. L'oxalate perhydrate, Na2C2O4.H2O2

Abstract
The vibrational spectra of the addition compound Na2C2O4.H2O2 show mutual exclusion of all the fundamentals in infrared (i.r.) and Raman. This feature is confirmed by a study of the partly deuterated compound. It agrees with the conclusion of a previous X-ray and nuclear magnetic resonance study that the hydrogen peroxide molecule in that crystal is planar and centrosymmetric. The two component molecules are held together by strong (9 kcal mole−1) hydrogen bonds. Some 20 lattice modes were detected in i.r. or Raman. For comparison purposes, the lattice spectra of anhydrous sodium oxalate were also investigated.

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