Characterization of two sequential polytripeptides containing glycine and ethyl‐glutamate residues

Abstract
The polytripeptides poly(glu(OEt)‐gly‐gly) and poly(glu(OEt)‐glu(OEt)‐gly) have been synthesized and characterized using infrared linear dichroism, ultraviolet circular dichroism spectroscopy, and electron microscopy. Both polymers have been obtained in a cross β conformation with antiparallel chains, however, there appear to be significant differences in the stability of this conformation for the two polymers. Poly(glu(OEt)‐gly‐gly) has also been shown to exist in a 31 polyglycine II type helix in aqueous solution whereas films cast from this solution appear to be random. Finally this same polymer can be obtained in either a random or an extended form trifluoroacetic acid depending on the nature of the substrate used for film casting.

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